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TM B/SE Ttar(s) to Crunch now?
Or wait for actual CD first?
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No reason to, unless you have an immediate use for them with Crunch.
EDIT: Since people don't seem to understand what I'm saying here I'll elaborate. If your SE Tyranitars would provide more value to you right now by having Crunch, TM them. If they wouldn't provide immediate value, there's absolutely no reason to TM now.
I'm not sure how you'd read my post to talk anything about the general usefulness of Tyranitar with Crunch. Since we don't know how many OP has or whether they have enough of better Ho-Oh counters, it's hard to say anything except "refrain from doing anything hasty unless it provides immediate value for you".